The photoinduced isomerization of trans- and cis- azobenzene and the cis- trans photoisomerization of the furylfulgide were studied with a pump- probe setup. the detection of the ultrafast transient absorption fs was realized using supercontinuum ( sc) broadband probe pulses generated in sapphire or caf2. a study of the cross- phase modulation showed that the sc could be described as linearly chirped. the spectral structure of the gain- profile of xecl was found to strongly influence the spectral and temporal characteristics of amplified ultrashort light pulses. a simple model was used to numerically study both effects as a fs function of amplifier length and input pulse energy. the results are in good agreement with expts. with these data, the performance of a xecl amplifier was optimized for. lv 68 fs forschungsseminar für fortgeschrittene mo ( n. ) ; nächster termin: 17. ), kinderspitalgasse 15, hs2.
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